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Article 2024 · 7 citations

Supramolecular Modification of Graphene Sponge with a Porphyrin Derivative Enhances the Photothermal Conversion Efficiency of a Solar Steam Generator

Ercarikci, Elif, Gultekin, Demet Demirci, Topcu, Ezgi, Kudas, Zuleyha, Alanyalioglu, Murat, Kiransan, Kader Dagci

Abstract

Solar energy seems to be a promising solution for obtaining clean water from saltwater and wastewater. With the solar steam generator system, it is possible to effectively acquire clean water from wastewater with a low-cost, sustainable, and environmentally friendly approach. In this study, PRF/GGSM, prepared by modification of gradient graphene sponge material (GGSM) with porphyrin derivative supramolecules (PRF), was investigated as a photothermal material for solar steam generation. PRF/GGSM possessing graphene and PRF served as ideal solar thermal converters that could easily gather sunlight. This material owing to its microporous and gradient hydrophilic structure has achieved a solar thermal conversion efficiency of up to 92% under 1 sun, corresponding to the water evaporation rate of 3.8 kg h-1 m-2. Moreover, this study exhibited that PRF/GGSM can efficiently generate clean water from seawater, wastewater, and even concentrated acid and alkali solutions.

Keywords
solar energy clean water graphenesponge porphyrin gradient structure OXIDE DEVICE FILMS WATER FOAM
WoS Categories
Nanoscience & Nanotechnology Materials Science, Multidisciplinary
Sustainable Development Goals
Citation
Journal
ACS APPLIED MATERIALS & INTERFACES
Year
2024
Volume
16
Issue
45
Pages
61910-61920
ISSN
1944-8244
eISSN
1944-8252
DOI
10.1021/acsami.4c11299
WoS UID
WOS:001344922700001
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