Solution processed high aspect ratio ultra-long vertically well-aligned ZnO nano scintillators for potential X-ray imaging applications
Kurudirek, Sinem V., Kurudirek, Murat, Erickson, Anna, Hertel, Nolan, Sellin, Paul J., Tratsiak, Yauhen, Lawrie, Benjamin J., Melcher, Charles L., Summers, Christopher J.
We report the photon (PL), electron (CL) and X-ray (XEL) induced luminescence characteristics of high aspect ratio ultra-long (similar to 50 mu m) ZnO nanorods (NRs) and discuss the potential for fast X-ray detection based on the consistent and efficient visible emission (similar to 580 nm) from ZnO NRs. Nanostructured ZnO scintillators were rearranged to form a vertically well-aligned NR design in order to help light absorption and coupling resulting in luminescent and fast scintillation properties. The design of the nanorod array combines the key advantages of a low-cost growth technique together with environmentally friendly and widely available materials. A low temperature hydrothermal method was adopted to grow ZnO NRs in one cycle growth and their structural, optical and X-ray scintillation properties were investigated. The relatively short (similar to 10 mu m) ZnO NRs emitting in the near-band-edge region were found to be almost insensitive to X-rays. On the other hand, the higher XEL response of long ZnO NRs, which is a key parameter for evaluation of materials to be used as scintillators for high quality X-ray detection and imaging, along with a decay time response in the order of ns confirmed promising scintillation properties for fast and high-resolution X-ray detector applications.
- Journal
- SCIENTIFIC REPORTS
- Year
- 2024
- Volume
- 14
- Issue
- 1
- ISSN
- 2045-2322
- DOI
- 10.1038/s41598-024-61895-6
- WoS UID
- WOS:001265868800004